袁自冰

袁自冰，男，博士、華南理工大學環境與能源學院教授、碩士生導師、博士生導師。

基本介紹

• 中文名：袁自冰
• 畢業院校：香港科技大學
• 學位/學歷：博士
• 職業：教師
• 專業方向：大氣污染控制
• 任職院校：華南理工大學

人物經歷

1998.9 – 2002.7 北京大學理學學士（化學）

2002.9 – 2006.11 香港科技大學哲學博士（大氣環境科學）

2006.11 – 2015.11 香港科技大學博士後、副研究員、研究助理教授、霍英東研究院大氣研究中心經理

2015.12 – 華南理工大學教授

學術任職

2017年3月份入選“大氣污染成因與控制技術研究”重點專項視頻評審專家，經濟快速發展地區區域空氣品質改善國際系列學術會議重要組織者之一。

研究方向

研究方向概述：

近年來，由於一系列減排措施的推行，我國主要城市群大氣細顆粒物（PM2.5）污染得到一定程度的改善。然而，臭氧污染日益嚴重，引起政府和公眾的廣泛關注。國外的相關經驗表明，臭氧治理比PM2.5要困難的多，需要時間也長的多。我國現階段普遍採取的以PM2.5為導向的控制策略不能滿足臭氧控制的需求，在PM2.5達標後，我國主要城市群的大氣污染控制勢必轉移到以臭氧為防控重點上來。以長三角、珠三角等典型光化學活躍區近地面臭氧污染為研究核心，在反應性有機物排放特徵、臭氧非線性變化控制機制以及氣候變化背景下大氣氧化性演變對近地面臭氧污染影響等方向開展深入研究，具體為：

1. 大氣反應性有機物來源量化與校驗：

反應性有機物在大氣化學過程和臭氧生成中起至關重要的作用，但其排放特徵和化學轉化尚未得到充分研究。針對當前反應性有機物來源研究的兩個薄弱環節：活性組分測量和化學轉化過程校正，藉助源排放測量、排放模型和文獻調研等手段，完善長三角和珠三角地區反應性有機物重要排放源化學成分譜，特別是補充現有反應性有機物源譜中缺失的支鏈雅套烏漏烯烴、反應性醛類等關鍵活性組分，構建本地化的反應性有機物排放源資料庫；以2016年為基準年，構建中國東部地區高時空解析度的反應性有機物排放源清單；針對反應性有機物重要排放源，量化表征大氣中反應淚享性有機物從源到受體點的化學轉化過程，建立基於地面觀測、模型反演和衛星遙感的反應性組分來源校驗方法；並預估長三角和珠三角精慨糠地區反應性有膠少碑頁機物未來5~10年的排放趨勢。

2. 光化學活躍區臭氧非線性變化控制機制研究：

通過結合基於觀測模型、三維空氣品質模型和衛星遙感等三種技術手段，定量識別不同氣象條件下本地生成及區域傳輸對長三角和珠三角不同地區臭氧的相對貢獻，闡明不同地區臭氧及其前體物的非線性關係及其時空變化特徵，揭示不同氣象條件下VOC敏感、NOx敏感及過渡區的空間分布；利用長期衛星遙感資料闡明長三角和珠三角地區評判VOC敏感盛戶習、NOx敏感及過渡區的FNR標準，識別兩區域臭氧控制懂全拳機制的長期變化趨勢，探索臭氧生成的敏感區域劃分隨NOx及VOCs削減的變化規律，為遏制臭氧污染事件發生的頻率和強度以及制定中長期臭氧達標規劃提供科學依據。

3. 氣候變化背景下大氣氧化性演變對近地面臭氧污染影響研究：

臭氧防控通常需要數十年的時間，在這一時間尺度上氣候變化對臭氧污染的影響不可忽視。根據長三角和珠三角多站點長期監測結果，建立描述臭氧、NOx及環境溫度關係的概念模型，識別溫度對不同區域臭氧生成效率的影響；將溫度因素納入排放源清單動態體系，在不同環境溫度下對部分揮發性VOCs排放源譜進行現場採樣與分析，闡明溫度對揮發性VOCs排放特徵的影響；在本地化的三維空氣品質模型中套用納入溫度因素的動態排放源清單並對環境溫度進行擾動，揭示兩區域的臭氧氣候補償效應，建立溫度與臭氧前體物回響關係之間的函式關係，為不同氣候變化背景下兩區域制定臭氧控制策略提供科學依據。

學術成果

主持項目

1.國家自然科學基金委“中國大氣複合污染的成因、健康影響和應對機制”聯合重大研究計畫重點支持項目“氣候變化背景下光化學活躍區大氣氧化性演變對近地面臭氧污染的影響研究”（91644221），250萬元（直接費用），2017.1-2020.12

2.國家重點研發計畫“大氣污染成因與控制技術研究”試點專項項目課題“大氣反應性有機物來源量化與校驗”（2016YFC0202201），730萬元，2016.7-2020.6

3.上海市科委科研計畫重點項循漿燥目課題“上海市臭氧非線性變化控制機制研究”（16DZ204605），70萬元，2016.7-2018.6

4.華南理工大學中央高校基本科研業務費重點項目“珠三角二次有機氣溶膠估算方法研究”，20萬元，2015.7-2017.6

學術論著

1.Zhao K, Luo H, Yuan Z, Xu D, Du Y, Zhang S, et al. Identification of close relationship between atmospheric oxidation and ozone formation regimes ina photochemically active region. Journal of Environmental Sciences 2021; 102:373-383.

2.Yang L, Yuan Z, Luo H, Wang Y, Xu Y, Duan Y, et al. Identification of long-term evolution of ozone sensitivity to precursors based on two-dimensional mutual verification. Science of The Total Environment 2020.

3.Luo H, Yang L, Yuan Z, Zhao K, Zhang S, Duan Y, et al. Synopticcondition-driven summertime ozone formation regime in Shanghai and the implication for dynamic ozone control strategies. Sci Total Environ 2020; 745:141130.

4..Yang L, Luo H, Yuan Z, Zheng J, Huang Z, Li C, et al. Quantitativeimpacts of meteorology and precursor emission changes on the long-term trend of ambient ozone over the Pearl River Delta, China, and implications for ozone control strategy. Atmospheric Chemistry and Physics 2019; 19: 12901-12916.

5.Xue J, Yu X, Yuan ZB, Griffith SM, Lau AKH, Seinfeld JH, et al.Efficient control of atmospheric sulfate production based on three formation regimes. Nature Geoscience 2019; 12: 977-+.

6. Huang, Z.J., Hu, Y.T., Zheng, J.Y.*, Yuan, Z.B., Russell, A.G.*, Ou, J.M. and Zhong, Z.M. A new combined stepwise-based high-order decoupled direct and reduced-form method to improve uncertainty analysis in PM2.5 simulations, Environmental Science and Technology, 2017, 51, 3852-3859.

7. Zhong, Z.M., Sha, Q.E., Zheng, J.Y.*, Yuan, Z.B., Gao, Z.J., Ou, J.M., Zheng, Z.Y., Li, C. and Huang, Z.J. Sector-based VOCs emission factors and source profiles for the surface coating industry in the Pearl River Delta region of China, Science of the Total Environment, 2017, 583, 19-28.

8. Yin, X.H., Huang, Z.J., Zheng, J.Y.*, Yuan, Z.B., Zhu, W.B., Huang, X.B. and Chen, D.H. Source contributions to PM2.5 in Guangdong province, China by numerical modeling: results and implications, Atmospheric Research, 2017, 186, 63-71.

9. Ou, J.M., Yuan, Z.B.*, Zheng, J.Y.*, Huang, Z.J., Shao, M., Li, Z.K., Huang, X.B., Guo, H. and Louie, P.K.K. Ambient ozone control in a photochemically active region: short-term despiking or long-term attainment?, Environmental Science and Technology, 2016, 50, 5720-5728.

10. Xue, J., Yuan, Z.B., Griffith, M., Yu, X., Lau, A.K.H. and Yu, J.Z.* Sulfate formation enhanced by a cocktail of High NOx, SO2, particulate matter, and droplet pH during haze-fog events in megacities in China: an observation-based modeling investigation, Environmental Science and Technology, 2016, 50, 7325-7334.

11. Li, C., Yuan, Z.B., Ou, J.M., Fan, X.L., Ye, S.Q., Xiao, T., Shi, Y.Q., Huang, Z.J., Ng, S.K.W., Zhong, Z.M. and Zheng, J.Y.* An AIS-based high-resolution ship emission inventory and its uncertainty in the Pearl River Delta region, China, Science of the Total Environment, 2016, 573, 1-10.

12. Lin, C.Q., Li, C.C.*, Lau, A.K.H., Yuan, Z.B., Lu, X.C., Tse, K.T., Fung, J.C.H., Li, Y., Yao, T. and Su, L. Assessment of satellite-based aerosol optical depth using continuous lidar observation, Atmospheric Environment, 2016, 140, 273-282.

13. Yin, S.S., Zheng, J.Y.*, Lu, Q., Yuan, Z.B., Huang, Z.J., Zhong, L.J. and Lin, H. A refined 2010-based VOC emission inventory and its improvement on modeling regional ozone in the Pearl River Delta region, China, Science of the Total Environment, 2015, 154, 426-438.

14. Li, Z.Y., Yuan, Z.B.*, Lau, A.K.H. and Louie, P.K.K. Characterization and source apportionment of health risks from ambient PM10 in Hong Kong over 2000-2011, Atmospheric Environment, 2015, 122, 892-899.

15. Su, L., Yuan, Z.B.*, Fung, J.C.H. and Lau, A.K.H. A comparison of HYSPLIT backward trajectories generated from two GDAS datasets, Science of the Total Environment, 2015, 506-507, 527-537.

16. Lin, C.Q., Li, Y.*, Yuan, Z.B., Lau, A.K.H., Li, C.C. and Fung, J.C.H. Using satellite remote sensing data to estimate the high-resolution distribution of ground-level PM2.5, Remote Sensing of Environment, 2015, 56, 117-128.

17. Huang, Z.J., Wang, S.S., Zheng, J.Y.*, Yuan, Z.B., Ye, S.Q. and Kang, D.W. Modeling inorganic nitrogen deposition in Guangdong province, China, Atmospheric Environment, 2015, 109, 147-160.

18. Yin, S.S., Zheng, J.Y.*, Lu, Q., Yuan, Z.B., Huang, Z.J., Zhong, L.J. and Lin, H. A refined 2010-based VOC emission inventory and its improvement on modeling regional ozone in the Pearl River Delta region, China, Science of the Total Environment, 2015, 154, 426-438.

19. Xue, J., Yuan, Z.B.*, Yu, J.Z. and Lau, A.K.H. An observation-based model for secondary inorganic aerosols, Aerosol and Air Quality Research, 2014, 14, 862-878.

20. Xue, J., Yuan, Z.B., Lau, A.K.H. and Yu, J.Z.* Insights into factors affecting nitrate in PM2.5 in a polluted high NOx environment through hourly observations and size distribution measurements, Journal of Geophysical Research-Atmospheres, 2014, 119, 4888-4902.

21. Yu, X., Yuan, Z.B., Fung, J.C.H., Xue, J., Li, Y., Zheng, J.Y. and Lau, A.K.H.* Ozone changes in response to the heavy-duty diesel truck control in the Pearl River Delta, Atmospheric Environment, 2014, 88, 269-274.

22. Yuan, Z.B., Yadav, V., Turner, J.R., Louie, P.K.K. and Lau, A.K.H.* Long-term trends of ambient particulate matter emission source contributions and the accountability of control strategies in Hong Kong over 1998-2008, Atmospheric Environment, 2013, 76, 21-31.

23. Yuan, Z.B., Zhong, L.J., Lau, A.K.H.*, Yu, J.Z. and Louie, P.K.K. Volatile organic compounds in the Pearl River Delta: Identification of source regions and recommendation for emission-oriented monitoring strategies, Atmospheric Environment, 2013, 76, 162-172.

24. Zhong, L.J., Louie, P.K.K.*, Zheng, J.Y., Wai, K.M., Ho, J.W.K., Yuan, Z.B., Lau, A.K.H., Yue, D.L. and Zhou, Y. The Pearl River Delta regional air quality monitoring network– regional collaborative efforts on joint air quality management, Aerosol and Air Quality Research, 2013, 13, 1582-1597.

25. Deng, X.J.*, Wu, D., Yu, J.Z., Lau, A.K.H., Li, F., Tan, H.B., Yuan, Z.B., Ng, W.M., Deng, T., Wu, C. and Zhou, X.J. Characterization of secondary aerosol and its extinction effects on visibility over the Pearl River Delta Region, China, Journal of Air and Waste Management Association, 2013, 63, 1012-1021.

26. Zhong, L.J., Louie, P.K.K.*, Zheng, J.Y., Yuan, Z.B., Yue, D.L., Ho, J.W.K. and Lau, A.K.H. Science-policy interplay: Air quality management in the Pearl River Delta and Hong Kong, Atmospheric Environment, 2013, 76, 3-10.

27. Lu, Q., Zheng, J.Y.*, Ye, S.Q., Shen, X.L., Yuan, Z.B. and Yin, S.S. Emission trends and source characteristics of SO2, NOx, PM10 and VOCs in the Pearl River Delta region from 2000 to 2009, Atmospheric Environment, 2013, 76, 11-20.

28. Louie, P.K.K.*, Ho, J.W.K., Tsang, R.C.W., Blake, D.R., Lau, A.K.H., Yu, J.Z., Yuan, Z.B., Wang, X.M., Shao, M. and Zhong, L.J. VOCs and OVOCs distribution and control policy implications in Pearl River Delta region, China, Atmospheric Environment, 2013, 76, 125-135.

29. Li, Y.C., Yu, J.Z.*, Ho, S.S.H., Schauer, J.J., Yuan, Z.B., Lau, A.K.H. and Louie, P.K.K. Chemical characteristics and source apportionment of fine particulate organic carbon in Hong Kong during high particulate matter episodes in winter 2003, Atmospheric Research, 2013, 120, 88-98.

30. Li, Y.C., Yu, J.Z.*, Ho, S.S.H., Yuan, Z.B., Lau, A.K.H. and Huang, X.F. Chemical characteristics of PM_2.5and organic aerosol source analysis during cold front episodes in Hong Kong, China, Atmospheric Research, 2012, 118, 41-51.

31. Zheng, J.Y.*, He, M., Shen, X.L., Yin, S.S. and Yuan, Z.B. High resolution of black carbon and organic carbon emissions in the Pearl River Delta region, China, Science of the Total Environment, 2012, 438, 189-200.

32. Lau, A.K.H., Yuan, Z.B.*, Yu, J.Z. and Louie, P.K.K. Source apportionment of ambient volatile organic compounds in Hong Kong, Science of the Total Environment, 2010, 408, 4138-4149.

33. Yuan, Z.B., Lau, A.K.H.*, Shao,M., Louie, P.K.K., Liu, S.C. and Zhu, T. Source analysis of volatile organic compounds by positive matrix factorization in urban and rural environments in Beijing, Journal of Geophysical Research, 2009, 114,doi:10.1029/2008JD011190.

34. Huang, X.F., Yu, J.Z.*, Yuan, Z.B., Lau, A.K.H. and Louie, P.K.K. Source analysis of high particulate matter days in Hong Kong, Atmospheric Environment, 2009, 43, 1196-1203.

35. Yuan, Z.B., Lau, A.K.H.*, Zhang, H.Y., Yu, J.Z., Louie, P.K.K. and Fung, J.C.H. Identification and spatiotemporal variation of dominant PM₁₀sources over Hong Kong, Atmospheric Environment, 2006, 40, 1803-1815.

36. Yuan, Z.B., Yu, J.Z.*, Lau, A.K.H., Louie, P.K.K. and Fung, J.C.H. Application of positive matrix factorization in estimating aerosol secondary organic carbon in Hong Kong and its relationship with secondary sulfate, Atmospheric Chemistry and Physics, 2006, 6, 25-34.

37. Huang, X.F., Yu, J.Z.*, He, L.Y. and Yuan, Z.B. Water-soluble organic carbon and oxalate in aerosols at a coastal urban site in China: Size distribution characteristics, sources and formation mechanisms, Journal of Geophysical Research, 2006, 111,doi:10.1029/2006JD007408.

38. Lo, J.C.F., Lau, A.K.H.*, Yuan, Z.B., Chen, F. and Fung, J.C.H. A physical modeling approach for identification of source regions of air pollutants, Atmospheric Chemistry and Physics Discussions, 2006, 6, 6467-6496.

39. Li, C.C., Mao, J.T.*, Lau, A.K.H., Yuan, Z.B., Wang, M.H. and Liu, X.Y. Application of MODIS satellite products to the air pollution research in Beijing, Science in China Series D– Earch Sciences, 2005, 48, Suppl. 2, 209-219.

40. Li, C.C., Mao, J.T.*, Lau, A.K.H., Chen, J.C., Yuan, Z.B., Liu, X.Y., Zhu, A.H. and Liu, G.Q. Characteristics of distribution and seasonal variation of aerosol optical depth in eastern China with MODIS products, Chinese Science Bulletin, 2003, 48, 2488-2495.

41. Fung, J.C.H.*, Lau, A.K.H., Lam, J.S.L. and Yuan, Z.B. Observational and modeling analysis of a severe air pollution episode in western Hong Kong. Journal of Geophysical Research, 2003, 110,doi: 10.1029/2004JD005105.

臭氧防控通常需要數十年的時間，在這一時間尺度上氣候變化對臭氧污染的影響不可忽視。根據長三角和珠三角多站點長期監測結果，建立描述臭氧、NOx及環境溫度關係的概念模型，識別溫度對不同區域臭氧生成效率的影響；將溫度因素納入排放源清單動態體系，在不同環境溫度下對部分揮發性VOCs排放源譜進行現場採樣與分析，闡明溫度對揮發性VOCs排放特徵的影響；在本地化的三維空氣品質模型中套用納入溫度因素的動態排放源清單並對環境溫度進行擾動，揭示兩區域的臭氧氣候補償效應，建立溫度與臭氧前體物回響關係之間的函式關係，為不同氣候變化背景下兩區域制定臭氧控制策略提供科學依據。

學術成果

主持項目

1.國家自然科學基金委“中國大氣複合污染的成因、健康影響和應對機制”聯合重大研究計畫重點支持項目“氣候變化背景下光化學活躍區大氣氧化性演變對近地面臭氧污染的影響研究”（91644221），250萬元（直接費用），2017.1-2020.12

2.國家重點研發計畫“大氣污染成因與控制技術研究”試點專項項目課題“大氣反應性有機物來源量化與校驗”（2016YFC0202201），730萬元，2016.7-2020.6

3.上海市科委科研計畫重點項目課題“上海市臭氧非線性變化控制機制研究”（16DZ204605），70萬元，2016.7-2018.6

4.華南理工大學中央高校基本科研業務費重點項目“珠三角二次有機氣溶膠估算方法研究”，20萬元，2015.7-2017.6

學術論著

1.Zhao K, Luo H, Yuan Z, Xu D, Du Y, Zhang S, et al. Identification of close relationship between atmospheric oxidation and ozone formation regimes ina photochemically active region. Journal of Environmental Sciences 2021; 102:373-383.

2.Yang L, Yuan Z, Luo H, Wang Y, Xu Y, Duan Y, et al. Identification of long-term evolution of ozone sensitivity to precursors based on two-dimensional mutual verification. Science of The Total Environment 2020.

3.Luo H, Yang L, Yuan Z, Zhao K, Zhang S, Duan Y, et al. Synopticcondition-driven summertime ozone formation regime in Shanghai and the implication for dynamic ozone control strategies. Sci Total Environ 2020; 745:141130.

4..Yang L, Luo H, Yuan Z, Zheng J, Huang Z, Li C, et al. Quantitativeimpacts of meteorology and precursor emission changes on the long-term trend of ambient ozone over the Pearl River Delta, China, and implications for ozone control strategy. Atmospheric Chemistry and Physics 2019; 19: 12901-12916.

5.Xue J, Yu X, Yuan ZB, Griffith SM, Lau AKH, Seinfeld JH, et al.Efficient control of atmospheric sulfate production based on three formation regimes. Nature Geoscience 2019; 12: 977-+.

6. Huang, Z.J., Hu, Y.T., Zheng, J.Y.*, Yuan, Z.B., Russell, A.G.*, Ou, J.M. and Zhong, Z.M. A new combined stepwise-based high-order decoupled direct and reduced-form method to improve uncertainty analysis in PM2.5 simulations, Environmental Science and Technology, 2017, 51, 3852-3859.

7. Zhong, Z.M., Sha, Q.E., Zheng, J.Y.*, Yuan, Z.B., Gao, Z.J., Ou, J.M., Zheng, Z.Y., Li, C. and Huang, Z.J. Sector-based VOCs emission factors and source profiles for the surface coating industry in the Pearl River Delta region of China, Science of the Total Environment, 2017, 583, 19-28.

8. Yin, X.H., Huang, Z.J., Zheng, J.Y.*, Yuan, Z.B., Zhu, W.B., Huang, X.B. and Chen, D.H. Source contributions to PM2.5 in Guangdong province, China by numerical modeling: results and implications, Atmospheric Research, 2017, 186, 63-71.

9. Ou, J.M., Yuan, Z.B.*, Zheng, J.Y.*, Huang, Z.J., Shao, M., Li, Z.K., Huang, X.B., Guo, H. and Louie, P.K.K. Ambient ozone control in a photochemically active region: short-term despiking or long-term attainment?, Environmental Science and Technology, 2016, 50, 5720-5728.

10. Xue, J., Yuan, Z.B., Griffith, M., Yu, X., Lau, A.K.H. and Yu, J.Z.* Sulfate formation enhanced by a cocktail of High NOx, SO2, particulate matter, and droplet pH during haze-fog events in megacities in China: an observation-based modeling investigation, Environmental Science and Technology, 2016, 50, 7325-7334.

11. Li, C., Yuan, Z.B., Ou, J.M., Fan, X.L., Ye, S.Q., Xiao, T., Shi, Y.Q., Huang, Z.J., Ng, S.K.W., Zhong, Z.M. and Zheng, J.Y.* An AIS-based high-resolution ship emission inventory and its uncertainty in the Pearl River Delta region, China, Science of the Total Environment, 2016, 573, 1-10.

12. Lin, C.Q., Li, C.C.*, Lau, A.K.H., Yuan, Z.B., Lu, X.C., Tse, K.T., Fung, J.C.H., Li, Y., Yao, T. and Su, L. Assessment of satellite-based aerosol optical depth using continuous lidar observation, Atmospheric Environment, 2016, 140, 273-282.

13. Yin, S.S., Zheng, J.Y.*, Lu, Q., Yuan, Z.B., Huang, Z.J., Zhong, L.J. and Lin, H. A refined 2010-based VOC emission inventory and its improvement on modeling regional ozone in the Pearl River Delta region, China, Science of the Total Environment, 2015, 154, 426-438.

14. Li, Z.Y., Yuan, Z.B.*, Lau, A.K.H. and Louie, P.K.K. Characterization and source apportionment of health risks from ambient PM10 in Hong Kong over 2000-2011, Atmospheric Environment, 2015, 122, 892-899.

15. Su, L., Yuan, Z.B.*, Fung, J.C.H. and Lau, A.K.H. A comparison of HYSPLIT backward trajectories generated from two GDAS datasets, Science of the Total Environment, 2015, 506-507, 527-537.

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